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The career, philanthropic, political, and personal aspects of Charles Richard Crane's life were closely intertwined. Among the correspondence of significance in the papers are letters to and from James Francis Abbott, Kathryn Newell Adams, Jane Addams, Edmund Henry Hynman Allenby, Edvard Benes, Boris III, King of Bulgaria, Louis Dembitz Brandeis, Nicholas Murray Butler, Frances F. Cleveland, Grover Cleveland, Archibald Gary Coolidge, Calvin Coolidge, John Dewey, Charles William Elliot, Hamlin Garland, William Rainey Harper, Jean-Jules Jusserand, William Lyon Mackenzie King, Alexander Kuprin, Robert Marion LaFollette, Seth Low, William Gibbs McAdoo, Jan Masaryk, Tomas Masaryk, Pavel Miliukov, John Pierpont Morgan, Alphonse Maria Mucha, Fridtjof Nansen, George Haven Putnam, John Davison Rockefeller Jr., Theodore Roosevelt, Upton Beall Sinclair, William Howard Taft, Lillian D. Wald, Herbert George Wells, Edith B. Wilson, Woodrow Wilson and other.

Papers include personal and professional correspondence, documents, manuscripts, photographs, drawings, printed materials. Most of the collection consists of Al'tschuler's personal and professional papers and letters from colleagues, patients and friends. Materials of the collection deal with professional affairs, revolution and civil war in Crimea, Al'tschuller's sanatorium in Yalta, emigration to Constantinople, Germany, Yugoslavia, Bulgaria, Czechoslovakia, activity of such organizations as Russkii zagranichnyi istoricheskii arkhiv and Vserossiiskii zemskii soiuz.

Correspondence, minutes of meetings, financial records, publications, notes, subject files, awards, speeches, reports and audiovisual materials document work by the Church Peace Union, its successors Council on Religion in International Affairs and Council on Ethics and International Affairs, and related organizations such as the World Alliance for International Friendship Through the Churches. The first installment of the CCEIA archival materials came to the RBML in 1974, with numerous additions over the years. A major addition in 1982 contained primarily the records of the Board of Directors and their semi-annual meetings, as well as the various programs and institutes of the Council, for the years 1972-1982, along with selected 1930s materials. 1986 addition contains presidential correspondence files, minutes of the Board of Trustees and committees, special projects, programs and conferences files, and the business and editorial files of "Worldview". Correspondents include John Foster Dulles, Jane Addams, Fiorello La Guardia, and Paul Tillich. 1990 and 2000 additions includes files of CCEIA presidents and vice presidents, paper and audiovisual materials on Merrill House Conversation Programs; Educational programs; International Monetary Fund/Lecture series; The Annals Of The Academy Of Political & Social Science; Washington Consultations; Colloquia for the Clergy; Church State Project; Asian Development & The Carribean Initiative; Korea: Year 2000 Project; fundraising files, printed materials and files of the Department of Publications.

This collection includes Papers of the Committee for the Education of Russian Youth in Exile, and its predecessors, Refugees in Russia and the Committee for the Rescue and Education of Russian Children, and Papers of the Committee' Director, Thomas Whittemore. The collection, which consists of correspondence, files on students supported by the Committee, financial records, photographs, manuscripts, documents, and printed materials, with the bulk dates 1914-1936.

Papers include typed carbons of correspondence, memoirs, speeches, and biographical materials. The correspondence consists of letters to and from Crane, 1869-1939, and telegrams and letters to his wife upon his death. The memoirs include information on his diplomatic service and travels. The speeches, 1910-1930, are largely based on his travels and activities. There are diaries by other persons of his trips to Albania, Russia in 1921, and to the Near East. Finally, biographical materials include editorials, articles, and speeches. While a sizable amount of material concerns Russia, the collection includes information on his other activities as well.

Collection of visiting cards of musical artists (composers, vocalists, conductors, etc.) and authors, presidents, and other celebrities of the 19th and 20th centuries, most bearing handwritten messages. There are also photographs and other memorabilia.