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The collection consists of correspondence, manuscripts, notes, photographs, subject files, and printed materials. Correspondents include Victor Chernov and George Kennan. Extensive notes by Mosely concern European diplomacy in the 1830s and the South Slavic Zadruga. There are thousands of photographs, chiefly from the Soviet Union ca. 1945-1955. Besides photographs of Soviet, Chinese, and East European political figures, such as Mao Tse-Tung, György Lukʹacs, and Boris Spasskiĭ, there are photographs of such Western figures as Enrico Berlinguer and Pablo Neruda. Subject files and mimeographed and printed materials include files on the Inter-University Committee on Travel Grants; papers on Soviet Studies distributed by St. Antony College, Oxford University; State Department research reports, and works by Mosely.

The collection of printed materials consists of eighteen boxes of newspaper clippings, oversize clippings and various newspaper letters and flyers. The clippings cover the 1920-1975 period and deal with topics including: World War II, Soviet affairs, the Korean War, the Vietnam War, Russian literature, Asian affairs and such individuals as Stalin, Khrushchev, Solzhenit︠s︡yn and Sakharov. There are newsletters from the St. Sergius High School and the Tolstoy Foundation as well as a number of pamphlets on East European affairs.

Papers of Stafford, reflecting a wide interest in psychedelic drugs, other drugs, and all aspects of the youth culture of the 1960s. Among the manuscript materials are drafts for chapters in his books, case histories, some correspondence, and materials showing the workings of the underground press. There are clippings, pamphlets, and books of both technical and popular interest.

The office files of the American Institute of Pacific Relations and the international Institute of Pacific Relations, containing correspondence and reports concerned with international conferences, research programs, and publications programs of both Institutes, and relating to the political, economic, and social problems in eastern and southern Asia and the South Pacific, as well as with problems of American foreign policy. There are many travel letters and on-the-spot reports relating to conditions in China, Japan, Russia, Australia, the Philippines, India, and Pakistan during the period 1933 to 1954.

The Tharchin Collection consists primarily of correspondence, publications and drafts, photographs, daybooks and financial accounts, and autobiographical materials. The geographic coverage of the collection spans both sides of the Himalayas, in particular, the activities of intellectuals, officials, missionaries, and other historical figures in India, Sikkim, and Tibet.

The reports and correspondence relating to UNRRA were arranged according to the nine administrative divisions of that organization that generated the documents: Bureau of Administration (26 reels); Office of the Diplomatic Adviser (4 reels); Office of the Director General (20 reels); Office of the Economic Adviser (4 reels); Office of Far Eastern Affairs (9 reels); Office of the General Counsel (19 reels); Office of the Historian (16 reels); Office of Public Information (1 reel); and Secretariat Executive Office (3 reels). Within each division, subsidiary bodies are typically separated into subject and country files.

These files have been compiled by the Rare Book and Manuscript Library from its origin in 1930 through the present day. The material derives largely from gifts, and the occasional purchase; much of the subject file in particular is made of ephemera included in the American Type Founders, Co. Library, purchased in 1942. Prospectuses and information sent by fine presses and book artists are added to the relevant files in an ongoing fashion. The files cover subjects from the beginning of printing to the current day.