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The Chinese Diary Collection contains 850 volumes of hardbound and softbound diaries, dating from 1930s to 1980s. Some volumes are filled with writing from cover to cover; some, partially filled; and some, with brief inscriptions. It includes 81 volumes by different individuals of Republican Period (1912-1949) and 95 small volumes penned by an engineer, with scientific data and personal contents. The contents recorded in the dairies are significant, for instance, a set of 20 work diaries by a mid-rank public security cadre member during and after the Cultural Revolution offers detailed history of public security operations for two decades. A set of 10 work diaries by an officer working in a ministry of the State Council in the 1980s documented the political and daily lives before and after the Tiananmen Massacre in association with the students' pro-democracy movement.

Interviews document the lives of seventeen prominent figures in the Republic of China (1911-1949). Narrators discuss military affairs, politics, national and regional governance, education, economics, culture, transportation, and other topics. Military campaigns are a major topic of the collection. Narrators discuss the operations and impacts of the Northern Expedition (1928-2928), Second Sino-Japanese War/War of Resistance (1937-1945), and Chinese Civil War (1945-1949). Narrators discuss the practical matters of governing during a period of upheaval. They also discuss the politics of the era and entities such as the Kuomintang and Chinese Communist Party. Many narrators studied abroad in the United States and Europe. The collection gives insights into Chinese education and the experiences of Chinese nationals abroad, including observations from their travels. Several narrators worked as diplomats for the Republican government and offer insights into international affairs and world leaders of the mid-20th century.

The Ephemera collection on Chinese science, technology, law, and society (中国科技法律社会汇集) contains over 800 items published in China, dating from circa 1906 to 2010, with its bulk dating from 1931 to 1981. Materials include pamphlets, handbooks, picture books, posters, lantern slides, literacy flash cards, etc. The subject areas of the materials include science, technology, agriculture, personal hygiene, economy, culture, law, society, and politics, etc. The collection also includes works that reflected social, political, industrial transformation in China.

The collection consists of correspondence, manuscripts, notes, photographs, subject files, and printed materials. Correspondents include Victor Chernov and George Kennan. Extensive notes by Mosely concern European diplomacy in the 1830s and the South Slavic Zadruga. There are thousands of photographs, chiefly from the Soviet Union ca. 1945-1955. Besides photographs of Soviet, Chinese, and East European political figures, such as Mao Tse-Tung, György Lukʹacs, and Boris Spasskiĭ, there are photographs of such Western figures as Enrico Berlinguer and Pablo Neruda. Subject files and mimeographed and printed materials include files on the Inter-University Committee on Travel Grants; papers on Soviet Studies distributed by St. Antony College, Oxford University; State Department research reports, and works by Mosely.