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The Chen Lifu papers (陳立夫檔案) mainly document his involvement in Chinese politics during the Republican era, dating from 1926 to 1989, with the bulk dates from 1926 to 1951. The papers consist of correspondence, portrait, meeting documents, reports, plans, speeches, writings, memoir, and printed materials. The papers focus on Chen Lifu's political career as the Head of the Central Bureau of Investigation and Statistics and the Minister of Education, as well as his general involvement in politics dating from 1926 to 1949.

The Chinese oral history project collection (中國口述歷史項目檔案) provides a wealth of information on the development of the project and its interviews with eminent Chinese political figures abroad in the United States and Hong Kong from 1958 to 1980s. The completed interviews are described separately under the Chinese oral history project, while this collection provides context of creation for the interviews and additional historical documentation on interviewees. The highlights of the collection consist of the administrative subject files, correspondence, interview photographs and reports, transcript drafts, collected autobiographies and manuscripts, audio recording, and card files of names mentioned in the transcripts.

The Chiu Chung-wei correspondence consists of outgoing and incoming letters and telegrams from and to Chiu when he was the Secretary of the President serving under the Acting President, Li Zongren, from 1949 to 1950. Other materials also include newspaper clippings and memoranda.

The Shih-hui Hsiung (Shihui Xiong) papers consist of materials documenting Hsiung's life and political career from 1907 to 1974. The highlights of the papers are the manuscripts, which include six volumes of Hsiung's memoir, seven volumes of diaries over 43 years, and approximately 440 original handwritten speech scripts. The photographs and political and military affairs related documents focus on Hsiung's active involvement in the northeast region and abroad from 1930 to 1948. The papers overall consist of correspondence, calligraphy scrolls, diaries, a diploma, documents, letter books, manuscripts of published and unpublished works, maps, newspaper clippings, notes, oversize military notices, poems, photographs, photograph albums, reports, and other materials.

The V. K. Wellington Koo papers document the diplomatic legacy of Wellington Koo as a Chinese statesman and diplomat of the 20th Century. The papers primarily consist of materials collected during Koo's diplomatic career, relating to the Lytton Commission, 1932-1933; the League of Nations, 1931-1940; the United Nations, 1944-1946; his ambassadorships to France, 1932-1941; to Britain, 1941-1946; to the United States, 1946-1956; as the Senior Advisor to the Republic of China from 1956; and as the Judge on the International Court of Justice, 1957-1966. The materials include correspondence, diaries, memoranda, manuscripts, documents, notes, speeches, maps, photographs, printed material, and audio visual material. The bulk of the materials emphasizes China's domestic and foreign affairs, such as the Sino-Japanese conflict, World War II and the Cold War in the Far East region, as well as the League of Nations and the United Nations.

The Yu Feng Tse papers (于鳳至檔案) document her family life and that of her spouse, the Young Marshall Zhang Xueliang, who was under house arrest since 1937, first in mainland China and later in Taiwan until he was free in 1992. The materials primarily consist of correspondence, writings, printed materials, photographs, as well as memorabilia, dating from 1928 to 2011, with its bulk dating from 1943 to 1996. The materials show the relationship between Yu Feng Tse who was in the United States and Zhang Xueliang who was in Taiwan at the time.