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The V. K. Wellington Koo papers document the diplomatic legacy of Wellington Koo as a Chinese statesman and diplomat of the 20th Century. The papers primarily consist of materials collected during Koo's diplomatic career, relating to the Lytton Commission, 1932-1933; the League of Nations, 1931-1940; the United Nations, 1944-1946; his ambassadorships to France, 1932-1941; to Britain, 1941-1946; to the United States, 1946-1956; as the Senior Advisor to the Republic of China from 1956; and as the Judge on the International Court of Justice, 1957-1966. The materials include correspondence, diaries, memoranda, manuscripts, documents, notes, speeches, maps, photographs, printed material, and audio visual material. The bulk of the materials emphasizes China's domestic and foreign affairs, such as the Sino-Japanese conflict, World War II and the Cold War in the Far East region, as well as the League of Nations and the United Nations.

The William Henry Donald letters primarily consist of correspondence between William Henry Donald (1875- 1946) and his friend, Harold K. Hochschild (1892-1981) where he described about his work in China, his involvement in the Xi'an Incident, and his life later in the Pacific Islands and return to China. Other materials in the collection include biographical information, a sketch of Donald, and news clippings about Donald.

The Yu Feng Tse papers (于鳳至檔案) document her family life and that of her spouse, the Young Marshall Zhang Xueliang, who was under house arrest since 1937, first in mainland China and later in Taiwan until he was free in 1992. The materials primarily consist of correspondence, writings, printed materials, photographs, as well as memorabilia, dating from 1928 to 2011, with its bulk dating from 1943 to 1996. The materials show the relationship between Yu Feng Tse who was in the United States and Zhang Xueliang who was in Taiwan at the time.