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The collection of historical photographs and lithographs of New York City consists of about 3,000 items dated from the 1850s until the 1980s. The collection is made up of color photographic prints, color negatives, black-and-white photographic prints, black-and-white negatives, copy prints, studio and cabinet cards, stereo cards, cyanotypes, albumen prints, gelatin silver prints, lantern slides, glass negatives, and Polaroid prints, lithographs, woodcuts, tear sheets, and engravings. The collection also includes official images, newspaper images, and candid images. Also included are images from the photo morgue of the New York Herald-Tribune newspaper, which ceased publication in 1966. Other images were purchased as copies from New-York Historical Society, Museum of the City of New York, WNYC-FM Radio, the Bettman Archive, and from collectors, private vendors, and other institutions. Photos by noted photographers are included.

Correspondence, manuscripts, original political cartoons, printed and photostatic materials relating to the political and social activities of the Society of Tammany, or Columbian order. Most of the correspondence is concerned with the formation of the Kilroe Tammaniana Collection, Kilroe's collection of books, documents, manuscripts, posters, cartoons, etc. relating to Tammany Hall. Also, letters from various members of the Tammany organization. The manuscripts include typescripts of Kilroe's works such as A COMPLETE BIBLIOGRAPHY OF SAINT TAMMANY and TAMMANY HALL AND THE TAMMANY SOCIETIES IN THE UNITED STATES. In addition there are manuscript and typescript records of various Tammany Societies with particular emphasis on the New York City Society and the New York County Democratic Party organization. Among the cartoons are 22 by John Tinney McCutcheon (1870-1949), over half of which deals with Tammany and New York politics while the remainder concerns national politics with an emphasis on presidential campaigns.

Correspondence, memoranda, and legal and financial documents of Keppel. The files deal largely with Keppel's personal and professional life during his tenure as President of the Carnegie Corporation, and also include some files from his years as Newton D. Baker's Third Assistant Secretary of War, and as Dean of Columbia College. There are extensive files of correspondence from and to Keppel's parents and children, as well as files concerning his activities in organizations such as the Century and Columbia University Clubs. The letters from friends and business associates concern American education, politics, business, and cultural life, particularly in the New York metropolitan area, from 1900 to 1943.