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This collection includes nine letters of Ralph Waldo Emerson as well as letters of Louis Agassiz, Amos Bronson Alcott, Oliver Wendell Holmes, Sr., Henry Wadsworth Longfellow, James Russell Lowell, John Lothrop Motley, Charles Sumner, and John Greenleaf Whittier. In addition, there are two incomplete manuscripts by Emerson and one document from the Liverpool Custom-house signed by Nathaniel Hawthorne as Consul for the United States. The collection also includes the corrected typescript, index, and page and galley proofs for Thomas Franklin Currier, A BIBLIOGRAPHY OF OLIVER WENDELL HOLMES (New York, 1953) which was edited by Professor Tilton. Also, some early correspondence and photographs of the Tilton family and friends. There are letters from the actors Annie Louise Ames, Richard J. Dillon, and Hans L. Meery to Tilton's grandfather, Bernard Paul Verne, as well as photographs, tintypes, and daguerreotypes of the Verne family and friends.

Correspondence, manuscripts, documents, photographs, memorabilia and printed materials of John Mitchel, John Purroy Mitchel, and other members of the Mitchel and Purroy families. The collection concerns Irish nationalism, family matters, Purroy family business interests in Central America, the John Purroy Mitchel Memorial and William Brown Meloney's files relating to his research and writing of "The Story of John Purroy Mitchel" along with the manuscript and typescript drafts for this unpublished biography.