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The Chen Lifu papers (陳立夫檔案) mainly document his involvement in Chinese politics during the Republican era, dating from 1926 to 1989, with the bulk dates from 1926 to 1951. The papers consist of correspondence, portrait, meeting documents, reports, plans, speeches, writings, memoir, and printed materials. The papers focus on Chen Lifu's political career as the Head of the Central Bureau of Investigation and Statistics and the Minister of Education, as well as his general involvement in politics dating from 1926 to 1949.

The H. H. Kung papers document Dr. Kung's political career from 1936 to 1944. The bulk of the papers consist of correspondence and political documents during the time when he was serving as the Minister of Finance, the Governor of the Central Bank of China, and the Vice Premier of the Executive Yuan. Materials in the collection include correspondence, writings, speeches, documents, reports, and telegrams relating to the Xi'an Incident, Sino-Japanese War, financial situation in China during the war year, his involvement in foreign diplomacy, Executive Yuan, the KMT Central committee, etc.

The Huang Fu papers consist of materials relating to Huang Fu's political involvement in the early revolutions, the Coup d'etat of 1924, the Nanking Incident, the Jinan Incident, the Tanggu Truce settlement and its aftermath, dating mostly from 1913 to 1945. Materials included in the papers are correspondence, documents, letters, telegrams, speeches and writings.

The Shih-hui Hsiung (Shihui Xiong) papers consist of materials documenting Hsiung's life and political career from 1907 to 1974. The highlights of the papers are the manuscripts, which include six volumes of Hsiung's memoir, seven volumes of diaries over 43 years, and approximately 440 original handwritten speech scripts. The photographs and political and military affairs related documents focus on Hsiung's active involvement in the northeast region and abroad from 1930 to 1948. The papers overall consist of correspondence, calligraphy scrolls, diaries, a diploma, documents, letter books, manuscripts of published and unpublished works, maps, newspaper clippings, notes, oversize military notices, poems, photographs, photograph albums, reports, and other materials.

The Ta-Chun Hsu papers (徐大春檔案) document his personal life and provide a glimpse of his career in China and in the United States. The bulk of the papers consist of correspondence related to his family and his personal life as a Chinese-American and an immigrant living in New York. The correspondence also highlights his relation to a prominent Chinese educator and philosopher, Hu Shih (胡適) and his family. There are also materials related to his father, Hsu Singloh (徐新六), who was a major finance and banking leader during the Second Sino-Japanese War. Also included are immigration and travel documents of T.C. Hsu. Other materials also include news clippings, articles, financial records, printed materials, portraits and photographs, maps and postcards.

The V. K. Wellington Koo papers document the diplomatic legacy of Wellington Koo as a Chinese statesman and diplomat of the 20th Century. The papers primarily consist of materials collected during Koo's diplomatic career, relating to the Lytton Commission, 1932-1933; the League of Nations, 1931-1940; the United Nations, 1944-1946; his ambassadorships to France, 1932-1941; to Britain, 1941-1946; to the United States, 1946-1956; as the Senior Advisor to the Republic of China from 1956; and as the Judge on the International Court of Justice, 1957-1966. The materials include correspondence, diaries, memoranda, manuscripts, documents, notes, speeches, maps, photographs, printed material, and audio visual material. The bulk of the materials emphasizes China's domestic and foreign affairs, such as the Sino-Japanese conflict, World War II and the Cold War in the Far East region, as well as the League of Nations and the United Nations.