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Correspondence and manuscripts of Van Doren, consisting of letters, poems, short stories, novels, plays, radio broadcast transcripts ("Invitation to Learning"), diaries, critical works, proofs, and printed works. Correspondents include Louise Bogan, Philip Booth, Babette Deutsch, Richard Eberhart, T.S. Eliot, John Gould Fletcher, Herbert Gorman, E.W. Howe, Robinson Jeffers, Archibald MacLeish, Louis MacNeice, Edgar Lee Masters, Lewis Mumford, Hyam Plutzik, Allen Tate, and Louis Zukovsky. Also, extensive correspondence with Robert Lax and Thomas Merton, as well as manuscripts by these two authors.

Scripts of plays that were presented during Smith's tenure as Director of the Brander Matthews Theater. Also, ca. 400 loose scrapbook leaves of mounted clippings, programs, and other memorabilia relating to the various theatrical productions with which Smith was associated. Many of these productions were produced by Columbia Theatre Associates.