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The collection includes two diaries of his American tour (one is made up of his rough travel notes, the other is in edited form for circulation), a memorial volume of manuscripts about his wife (Ann Loxley Rhees) prepared by his daughter Eliza (Mrs. Nicholas Murray), and 1851 passport of Nicholas Murray, a letter of Thomas Chalmers Murray to his sister Mary Jones Murray Butler (the mother of Nicholas Murray Butler, President of Columbia University), correspondence between Welsh historian Gwyn A. Williams and collection donor Mary Butler Brown, an essay entitled "Morgan John Rhees and Beula" by Gwyn A. Williams, Ann Loxley Rhees's valedictory oration on graduation from Philadelphia's Ladies Academy, an address on female education ca. 1789, family obituary clippings, poems, misc. items, and a photograph of Ann Loxley Rhees. An edited version of substantial sections of the diaries of M.J. Rhees was published in John Thomas Griffith's 1910 biography and miscellany of Rhees and his family, a copy of which is included in this collection. An edited version of a previously unpublished section of the diary, from May 2nd to July 9th 1795, was published in Northwest Ohio History (vol. 80, no. 2), but it is an unreliable transcription containing many inaccuracies, according to Dr E. Wyn James of Cardiff University, who is working on a new edition of the M.J. Rhees diaries.

An artificial collection of phonograph records, reels of audio tape recordings, and motion picture films recording a variety of Columbia University academic and extra-curricular activities and events such as lectures; speeches, some at award ceremonies; commencement; installation of Nicholas M. Butler and Dwight D. Eisenhower as presidents of the university; King George VI of England during his visit, 1939; speech of England's Queen Mother, Elizabeth in 1954; homecoming; football, the band; academic and alumni conferences; and radio programs under the auspices of Columbia. Many of the recordings are of Eisenhower. Other prominent personalities include John Foster Dulles, Herbert Hoover, Isidor Rabi, Eleanor Roosevelt, John R. Dunning, and the Shah of Iran.

Correspondence, research notes, articles, clippings, photostats, and photographs. These files concern his interest in Pierre Bayle, Antoine Arlier, and the Renaissance in Provence, as well as the Romanic Review, philology, French, Spanish, and celtic studies. Among the correspondents are: Philippe Berthelot, Nicholas Murray Butler, F.R. Coudert, John H. Finley, the Prince de Ligne, Curtis Hidden Page, William B. Parsons, and Aime ́Puech.

This collection includes a very small number of personal papers from Ware; photographs of students, faculty, and school buildings, 1880s-1920s; memorials and testimonials to Ware; and miscellaneous clippings (including clippings of articles about Marcia Mead, first woman graduate of the School of Architecture), invitations (including two invitations to the first commencement of the University of the City of New York, 1834), greeting cards and announcements.

A significant and sizeable archive of primary materials relating to the career of Charles A. Beard, compiled in the 1970s by Miriam (Beard) Vagts and William Beard. The collection includes more than 300 original letters, manuscripts, and printed material.