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The Union Settlement Association Records document a century of the settlement's activities, and provide a unique view of the first wave of the settlement movement in America. They document social conditions, demographic change, political activity, philanthropy and social work in East Harlem with a strong emphasis on the urban renewal period of the 1950s and '60s. The records include: annual reports, board minutes and committee files, headworker and executive director files, program reports, community organization files, and visual materials such as photographs, maps and architectural drawings.

The collection consists of the editorial and production archives of Vanguard Press: correspondence, manuscripts, contracts, memoranda, galley proofs, photographs, clippings, and printed materials. The correspondence and editorial files contain a wealth of detailed information about individual authors and the growth and development of the Press. Among the cataloged correspondents are: Nelson Algren, Saul Bellow, Stephen Vincent Benét, William Rose Benét; Phyllis Bottome; Pierre Boulle; Jocelyn Brooke; Cyril Connolly; A.J. Cronin; Nigel Dennis; John Dewey; Max Eastman; James T. Farrell; Vardis Fisher; Richard Garnett; Theodor Seuss Geisel; Louis Golding; Paul Goodman; Horace Gregory; Geoffrey Grigson; Lillian Hellman; William Heyen; Harold L. Ickes; Christopher Isherwood; Alfred Kazin; Philip Lamantia; Sinclair Lewis; Emanuel Litvinoff; Dwight Macdonald; Archibald MacLeish; Marshall McLuhan; Thomas Mann; Edgar Lee Masters; H. L. Mencken; William Meredith; Joyce Carol Oates; Katherine Anne Porter; Barbara Pym; William Sansom; William Saroyan; Ramon J. Sender; Upton Sinclair; Rex Stout; Edith Sitwell; Paul Theroux; Lionel Trilling; Harry S. Trumam; Louis Untermeyer; Eudora Welty; Richard Wilbur; and Thornton Wilder. There are some manuscripts by Bellow; Bottome; Boulle; Farrell; Grigson; Litvinoff; MacDonald; Oates; John Cowper Powys; Arthur Schlesinger, Jr.; Patrick Tanner; William Targ; Theroux; and Sitwell.

The collection includes the original manuscript of "Surrender on Demand", Mr. Fry's account of his wartime experiences, which was later rewritten for young readers as "Assignment Rescue" (New York, Four Winds Press, 1968). Among the correspondents represented in the collection are Marc Chagall, Jacques Lipchitz, Roger Baldwin, Norman Thomas, J. Edgar Hoover, and Herman Wouk. In addition to the material relating to the Emergency Relief Committee (later known as the International Rescue Committee), the collection includes correspondence and papers concerning Fry's work as a writer on foreign affairs as well as copies of his books.

The collection consists of approximately 100 articles by Seni︠u︡tovich (often signed Seni︠u︡tovich-Berezhnyĭ) on topics including genealogy, heraldry, military history, the history of Russia and the Ukraine, and the Russian emigration. There is also correspondence both to and from Seni︠u︡tovich, newsletters from the Ukrainian Genealogical and Heraldic Society, an autobiographical essay by Seni︠u︡tovich, and three photographs.

Correspondence, manuscripts, notes and printed materials concerning Robinson's work at the University of Pennsylvania School of Social Work and her publications which include a memorial volume about her colleague, Jessie Taft.