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The Hung-Hsun Ling papers document Ling's life as a railway engineer and his contribution to the development of rail infrastructure in China during the Republican period. The papers include two manuscripts of his autobiographies and 14 photographs depicting him as an engineer taken during and after the construction of various railway projects in China and other locations dating from 1916 to 1965, as well as a portrait of him at age 80. The papers also include five books related to the history and the development of railways in China written in Chinese by Ling from 1954 to 1977.

The Ta-Chun Hsu papers (徐大春檔案) document his personal life and provide a glimpse of his career in China and in the United States. The bulk of the papers consist of correspondence related to his family and his personal life as a Chinese-American and an immigrant living in New York. The correspondence also highlights his relation to a prominent Chinese educator and philosopher, Hu Shih (胡適) and his family. There are also materials related to his father, Hsu Singloh (徐新六), who was a major finance and banking leader during the Second Sino-Japanese War. Also included are immigration and travel documents of T.C. Hsu. Other materials also include news clippings, articles, financial records, printed materials, portraits and photographs, maps and postcards.