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Minutes, correspondence, annual reports, press releases, financial records, photographs, memorabilia, audiovisual, digital and printed materials document the philanthropic activities and administration of the Carnegie Corporation of New York. The collection is actively growing, primarily through regular document transfers from the Carnegie Corporation of New York. Andrew Carnegie's biographical information and personal philanthropic activity can be found in Series VII. In addition, his pre-1911 gifts, most notably his donations for libraries and church organs, can be found on microfilm (Series II), in the Home Trust Company Records (VI.A), and Financial Record Books (I.C.1). Grant files (Series III.A), which comprise the bulk of the collection) provide information on projects and institutions founded, endowed or supported by the Corporation. The Special Initiatives series (Series IV) contains the records of task forces, commissions and councils, formed by the Corporation mostly during the 1970s, 1980s, and 1990s to address specific issues. The Corporation's records include those of other Carnegie philanthropic organizations (Series VI), including the Carnegie Foundation for the Advancement of Teaching and the Home Trust Company, both of which shared staff, officers, and office space with the Corporation for a period of time.

The correspondence, papers, and documents relating to Franklins' work in the fields of psychology and logic. The papers are mainly those of Christine Ladd Franklin. Among the selected autographs are fourteen letters from Henry Holt to Fabian Franklin and four letters from Bertrand Russell to Christine Ladd Franklin.

Many typescripts of Horton's lectures, research studies, articles, and professional case histories, material gathered by the Cartesian Research Bureau, and correspondence, chiefly professional. The correspondence is largely that of Samuel Dana Horton, father of Lydiard, and includes eight letters of Moreton Frewen, three each of Robert Todd Lincoln, John Fiske, and C.W. Fremantle, one of President James A. Garfield, and typescript copies of nine from Henry James. There are two letters from Dr. Horton to his guardian, Frederick W. Holls, and one each to Horton from William James and William Howard Taft. The remaining indexed correspondence is with colleagues and professional associates. Some of the case histories contain correspondence as well as documentary material. Also, a diary of Lydiard H. Horton for July to December 1896, and copies of excerpts from the diary of Samuel Dana Horton, 1860, photographs, newspaper clippings, and printed pamphlets.