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Three sketchbooks; the first, 1893-1894, containing sketches from his student years at the Columbia School of Mines, Department of Architecture (he received his degree in 1894); the second, 1894-1896, containing sketches made as a student at the Ecole des Beaux-Arts in Paris; and the third, circa 1896-circa 1905, containing sketches for a variety of projects and designs. Buildings and other structures depicted include the Academy of Music on 14th Street, New York City (a seating plan); Wells Fargo Bank Building, Portland, Oregon, 1910; Reunion Hall, Princeton University, 1902; lantern for the Aetna Building, Hartford, Connecticut; Woodland Street entrance to Kinney Park, Hartford, Connecticut, 1905 (some drawings are by others). Program notes from the classes of Paul Blondel and J. Gaudet at the Ecole des Beaux Arts are included. Also, designs (some done in partnership with Joseph Urban) for proposals for the Metropolitan Opera Company on various sites in New York City, circa 1920s; and designs for shopping and music centers in New York City, to 1936.

This collection primarily contains architectural renderings executed by Long in 1906 for a memorial issue of BUILDINGS magazine dedicated to New York architect Stanford White. These drawings represent White's most famous structures designed while he was a partner with McKim, Mead & White. Buildings depicted include Madison Square Garden, the New York Herald Building, and the Washington Memorial Arch, all in New York City, among others. Also included in this collection are miscellaneous architectural drawings by Long, Chester B. Price, and others, circa 1920s-1930s; and printed material.