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Minutes, correspondence, annual reports, press releases, financial records, photographs, memorabilia, audiovisual, digital and printed materials document the philanthropic activities and administration of the Carnegie Corporation of New York. The collection is actively growing, primarily through regular document transfers from the Carnegie Corporation of New York. Andrew Carnegie's biographical information and personal philanthropic activity can be found in Series VII. In addition, his pre-1911 gifts, most notably his donations for libraries and church organs, can be found on microfilm (Series II), in the Home Trust Company Records (VI.A), and Financial Record Books (I.C.1). Grant files (Series III.A), which comprise the bulk of the collection) provide information on projects and institutions founded, endowed or supported by the Corporation. The Special Initiatives series (Series IV) contains the records of task forces, commissions and councils, formed by the Corporation mostly during the 1970s, 1980s, and 1990s to address specific issues. The Corporation's records include those of other Carnegie philanthropic organizations (Series VI), including the Carnegie Foundation for the Advancement of Teaching and the Home Trust Company, both of which shared staff, officers, and office space with the Corporation for a period of time.

The letters and manuscripts of Keyser, including the notes and manuscripts for his lectures, essays, and books, as well as his correspondence with colleagues and mathematicians throughout the world. There are letters from Benjamin N. Cardozo, Alfred Korzybski, Anna Hempstead Branch, James Truslow Adams, and Clarence Day, Jr.

Professional and personal papers of Smith, including correspondence and manuscripts from his students, family, contemporary mathematicians and teaching colleagues about the history and teaching of mathematics, his many committees, administrative matters at Teachers College, and his travels and collecting. Also, the manuscripts of his writings and his notes.