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The collection consiste of correspondence, memoranda, reports, bulletins, clippings, photographs, awards, and printed material. The files, arranged by genre and topic and reflect her philanthropic and legislative work in the areas of health, specifically cancer, heart disease, and mental health. Her civic and legislative work is covered in detail, as well as her private interests and activities.

Personal, academic, and legal correspondence, manuscripts, documents, photographs, and memoranda. Among the legal files, there is particular emphasis on labor and welfare law. The files also contain materials about his judicial appointment, the American Law Institute, the Columbia University School of Law, and the Project on International Procedure. Among the major correspondents are: James A. Farley, Arthur J. Goldberg, Philip C. Jessup, Robert F. Kennedy, Harold R. Medina, James A. Pike, and Lionel Trilling

Correspondence and manuscripts. The collection includes manuscript drafts and typescripts of two volumes of his autobiography: THE OLD CENTURY AND SEVEN MORE YEARS, 1938; and THE WEALD OF YOUTH, 1942. There are also 13 volumes of early notebooks for the period 1894 until 1909 (from age 8 to 22) containing drafts of over 200 poems, 19 short stories and many drawings. There is some correspondence about the autobiography. Also includes 21 letters from Arnold Bennett, 51 letters from Lady Ottoline Morrell, 26 letters from H.M. Tomlinson, 19 letters from Sassoon to his mother-in-law, Lady Gatty, 22 letters from Sassoon to his son, letters from many others, and a typescript of his poem "A love affair" with holograph note

Letters written to Gay from political and literary contemporaries such as Horace Greeley, Charles Sumner, and William Bryant; reports in letter form from his reporters at the front during the Civil War; and personal correspondence including many letters from his wife, Elizabeth Neall Gay. Letters written to Mrs. Gay from family friends and business associates including many from her husband. Correspondence of other members of the Gay family including Walter Gay, Sarah Gay, and Allan Gay. Diaries, notebooks, and journals of Sydney Howard Gay.

Correspondence, manuscript, and printed materials of Kees. There are fourteen letters from Kees to Herbert Cahoon, twelve letters from James T. Farrell to Kees, the manuscript of Kees' THE LAST MAN, and announcements and clippings by and about Kees.