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Letters written to Gay from political and literary contemporaries such as Horace Greeley, Charles Sumner, and William Bryant; reports in letter form from his reporters at the front during the Civil War; and personal correspondence including many letters from his wife, Elizabeth Neall Gay. Letters written to Mrs. Gay from family friends and business associates including many from her husband. Correspondence of other members of the Gay family including Walter Gay, Sarah Gay, and Allan Gay. Diaries, notebooks, and journals of Sydney Howard Gay.

Correspondence, manuscripts, documents, photographs, memorabilia and printed materials of John Mitchel, John Purroy Mitchel, and other members of the Mitchel and Purroy families. The collection concerns Irish nationalism, family matters, Purroy family business interests in Central America, the John Purroy Mitchel Memorial and William Brown Meloney's files relating to his research and writing of "The Story of John Purroy Mitchel" along with the manuscript and typescript drafts for this unpublished biography.

Correspondence, manuscripts, typescripts, contracts, legal briefs, patents, and other documents, music scores, cartoons, technical drawings, account books, blueprints, photographs, clippings, printed legal briefs & transcripts, proofs, scrapbooks, and other printed materials of William M. Speer.