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Minutes, correspondence, annual reports, press releases, financial records, photographs, memorabilia, audiovisual, digital and printed materials document the philanthropic activities and administration of the Carnegie Corporation of New York. The collection is actively growing, primarily through regular document transfers from the Carnegie Corporation of New York. Andrew Carnegie's biographical information and personal philanthropic activity can be found in Series VII. In addition, his pre-1911 gifts, most notably his donations for libraries and church organs, can be found on microfilm (Series II), in the Home Trust Company Records (VI.A), and Financial Record Books (I.C.1). Grant files (Series III.A), which comprise the bulk of the collection) provide information on projects and institutions founded, endowed or supported by the Corporation. The Special Initiatives series (Series IV) contains the records of task forces, commissions and councils, formed by the Corporation mostly during the 1970s, 1980s, and 1990s to address specific issues. The Corporation's records include those of other Carnegie philanthropic organizations (Series VI), including the Carnegie Foundation for the Advancement of Teaching and the Home Trust Company, both of which shared staff, officers, and office space with the Corporation for a period of time.

Correspondence relating to Erskine's various educational, musical and literary interests; manuscripts of his writings; lecture notes for college courses; souvenirs of his army service in World War I and his Columbia University professorship, and student papers from his own school and college days. Also, biographical file, scrapbooks, and articles.

Personal and professional papers including correspondence, manuscripts, documents, diaries, journals, photographs, and printed materials relating to his teaching at various universities, his literary studies and writings, and his professional activities in such organizations as the Moder Language Association and P.E.N. His correspondents include contemporary authors such as Edmund Blunden, Christopher Hassall, Louis Kronenberger; scholars such as James P. Clifford, Leon Edel, and A.L. Rowse. There are also some letters collected by Halsband, including those by Mrs Piozzi, John Wilkes (1727-1797) and John Stuart, 3rd Earl of Bute (1713-1792). Among the manuscripts are notes, drafts, typescripts, and proofs of his LIFE OF LADY WORTLEY MONTAGU (Oxford, 1956) and COMPLETE LETTERS OF LADY MARY WORTLEY MONTAGU (Oxford, 1965-1967). Also, manuscripts and typescripts of Halsband's diaries, journals, lectures, articles, book reviews, and essays. The printed materials include ephemera, books, and offprints by Halsband and books by other authors inscribed to him. There is a watercolor portrait of Halsband by Stephen Andrews, London, ca. 1966.