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Correspondence of Williamson covering his college years and his positions at Bryn Mawr College, the New York Public Library, the Carnegie Foundation, and the Rockefeller Foundation. A significant portion of Williamson's Columbia University correspondence and memoranda is addressed to or related to Roger Howson, University Librarian from 1926 to 1940. The manuscripts, chiefly typescripts, are concerned with library science and educational topics. Also, clippings and pamphlet files with some related correspondence and typescripts dealing with education and particularly the use of television as a teaching aid.

Correspondence, notes, articles, reports, and speeches of Gildersleeve, including materials relating to the United Nations Conference in San Francisco, 1945, the Dumbarton Oaks Conference, the International Federation of University Women, the American Association of University Women, the American Council on Education, and the Near East College Association. The most note-worthy item in the collection is a letter from President Franklin D. Roosevelt, appointing Dean Gildersleeve to serve as a member of the U.S. Delegation to the Charter Conference of the United Nations. The collection also contains some material relating to Barnard College affairs.