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Minutes, correspondence, annual reports, press releases, financial records, photographs, memorabilia, audiovisual, digital and printed materials document the philanthropic activities and administration of the Carnegie Corporation of New York. The collection is actively growing, primarily through regular document transfers from the Carnegie Corporation of New York. Andrew Carnegie's biographical information and personal philanthropic activity can be found in Series VII. In addition, his pre-1911 gifts, most notably his donations for libraries and church organs, can be found on microfilm (Series II), in the Home Trust Company Records (VI.A), and Financial Record Books (I.C.1). Grant files (Series III.A), which comprise the bulk of the collection) provide information on projects and institutions founded, endowed or supported by the Corporation. The Special Initiatives series (Series IV) contains the records of task forces, commissions and councils, formed by the Corporation mostly during the 1970s, 1980s, and 1990s to address specific issues. The Corporation's records include those of other Carnegie philanthropic organizations (Series VI), including the Carnegie Foundation for the Advancement of Teaching and the Home Trust Company, both of which shared staff, officers, and office space with the Corporation for a period of time.

This collections contants the administrative papers from 1950 to 1970s, which document the establishment of the Assembly and how it operated in the framework of Columbia University and its Business School. It also includes the volumes created for each Assembly topic and meeting year. The volumes contain both original manuscript material (e.g., correspondence, memos, reports, photographs, programs, etc.) related to the planning and execution of each meeting as well as published reports and publications generated for the meeting. Topics addressed by the Assembly over the years include: US Foreign Policy, Outer Space, Nuclear/Atom Power, International Relations, Collapse of the USSR, Arms Control, US Economy, Domestic policy issues (health insurance, labor, black economic development), Religion and American Life, Social Issues, Arts and Public Policy, Environmental issues, Politics, Tax System, Financial Systems, World Migration and US Policy. The collection also includes The Assembly's publications and a participant index.