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Correspondence, manuscripts, playscripts, screenplays, diaries, documents, contracts, financial records, photographs, phonograph records, motion pictures, playbills, posters, sheet music, cartoons, art work, memorabilia, scrapbooks, and printed materials. . The collection consists chiefly of correspondence and production files relating to the creation, production, and performance of their works for stage, screen, radio, and television, such as Leave It To Me and Kiss Me Kate (with music by Cole Porter), Boy Meets Girl, and My Three Angels. Correspondence (with twentieth century authors, playwrights, musicians, political figures, and actors) includes: George Abbott, Jean Arthur, Bennett Cerf, Katharine Cornell, Jo Davidson, George and Ira Gershwin, Alec Guinness, W. Averell Harriman, Lilli Lehmann, Mary Martin, Laurence Olivier, Mary Pickford, Cole Porter, Regina Resnick, Eleanor Roosevelt, Robert E. Sherwood, Lincoln Steffens, Kurt Weill, Rebecca West, and Thornton Wilder. There is also correspondence concerning Bella Spewack's work with the New York Girls' Scholarship, UNRA, and the Sports Center of Israel. In addition to the production files, there are manuscripts and typescript drafts for novels, short stories, and articles by the Spewacks.

The records of W.R. Grace & Co. cover the rise of the Grace shipping business from 1864 until World War II. The early correspondence concerns all aspects of the shipping business in New York and South America, mining interests in Peru and Chile, the railroad in Costa Rica, the inter-ocean canal planned for Nicaragua, and political interests throughout Central and South America. There are letter books, correspondence, and scrapbooks of clippings for all aspects of W.R. Grace's career. There are minute books and other documents for more than 50 subsidiary companies owned by W.R. Grace & Co. or by family members. The papers of Joseph Peter Grace (1872-1950) continue the business, family, and philanthropic activities until 1942. There are also 20 reels of motion picture film about the Grace Co. South American interests in the 1950s.