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Drawings, prints, watercolors, photographs, and reproductions, largely undated (late 19th- through the 20th century) of architectural and other subjects by Harriman, with some by others including Perry Coke Smith, Howard J. Custer, and unidentified artists and architects. Of note is an undated unidentified photograph of late 19th- or early 20th-century art or architecture students.

Also, correspondence with Norman Bel Geddes, Monroe Biddle, John M. Blair, Harry T. Carman, Carolyn K. Christenson, Joseph S. Clarke, Jr., Thomas H. Creighton, Paul Cret, C.C. Cunningham, F.G. Fassett, Jr., Loring Dowst, John E. Harbeson, Oliver Hall, Jared C. Ingersoll, Gaylord P. Harnwell, William Fontaine Jones, Joseph Judge, William Lescaze, John D. Morse, William F. Paris, Charles E. Peterson, Ruth C. Roberts, Henry Shapiro, Oscar Stonorov, J.J. Sweeney, James M. Willcox, Owen J. Wister, Frank Lloyd Wright, Bruno Zevi, and others. This relates to proposed development of air rights over New York City's Pennsylvania Railroad Station, 1955; architectural projects in Pennsylvania relating to mental health, 1955; proposed new Independence Mall Building in Philadelphia, 1955; the 1954 Boston Art Festival Architectural Exhibit; sculpture committee on the design of the Ella Butt McManus monument, Connecticut, 1954-1955; the Philadelphia Saving Fund Society, building designed by Howe & Lescaze (with related memoranda, manuscripts of articles and talks, press releases, and architectural analyses), 1930-1939; and the Jefferson National Expansion Memorial, St. Louis (with related printed material, clippings, and photograph)

Miscellaneous architectural drawings and sketches. Also includes papers and clippings on Bronx County Court House and St. Paul's Chapel, Chicago.