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Letters written to Gouverneur Morris from many of his contemporaries including George Washington, Thomas Jefferson, Thomas Paine, John Paul Jones, Nathaniel Greene, Philip Schuyler, Robert Morris, George Plater, William Short, William T. Franklin, and Thomas Pinckney. Letters from Gouverneur Morris to George Washington, John Jay, Lafayette, Philip Schuyler, Nathaniel Greene, and others. Personal correspondence from Madame Foucault, John Parish, and others. Manuscripts and documents relating to events in which Morris was a participant or interested party such as the Genet Affair and the "Lost Million" Affair; diplomatic correspondence with French ministers of foreign affairs, 1792-1794, and miscellaneous articles and reports by Morris, many on public finance and economics.

Correspondence and papers of Vroom, consisting chiefly of letters received by Vroom from a variety of individuals including J.H. Austin, Andrew Deutcher, Alfred Gale, P.B. Kennedy, James Parker, and John M. Wycoff. These letters deal with business, legal, and political affairs. There are a few personal letters, various legal papers and documents, and memoranda written by Vroom. The early material contains Vroom family letters and documents including letters to Vroom's father, Peter D. Vroom (1745-1831). Also of interest is Vroom's Latin-English vocabulary notebook kept during his junior year at Columbia College, 1807. The notebook contains a list of his classmates. In addition there is his 1808 Columbia College Commencement address.

Correspondence and legal and business papers of Peter Van Schaack and his family. The collection includes letters to and from Egbert Benson, Henry Cruger, James Duane, William Laight, Theodore Sedgwick, Peter Silvester, John Vardill, and many others. The letters deal with such subjects as taxation, the siege of Boston, George Washington, Tories, the Jay Treaty, Shays' Rebellion, and the many prominent people with whom Van Schaack was acquainted, including the Jay family and Gouverneur Morris. There is a large number of letters to and from his brother, Henry Van Schaack (1733-1823). The correspondence contains many political and social opinions regarding America and England before, during, and after the Revolutionary War. Many of the legal documents concern the disputed claims to the Van Rensselaer properties in Claverack and Westenhook, N.Y., as well as land claims around Kinderhoek, N.Y. Henry Cruger Van Schaack added to the collection more letters from well-known people as well as legal and family papers. These are mostly dated in the mid-19th century, and deal in part with the Delaware and Hudson Canal Company, the Berkshire Iron Works, and similar business ventures. Many documents are Colonial-era deeds or concern early land disputes such as the New York-Massachusetts boundary dispute.