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Correspondence, memoranda, position papers, campaign materials, speeches, photographs, and printed materials relating primarily to Samuels' unsuccessful 1970 campaign for governor of New York. Included with the collection are campaign materials for other candidates, and campaign buttons for Samuels, Nelson A. Rockefeller, and others. Major correspondents include William Averell Harriman, Hubert Horatio Humphrey, LeRoi Jones, Edward I. Koch, John V. Lindsay, Robert Moses, and Edmund S. Muskie.

Correspondence, minutes, reports, documents, scrapbooks, publications, memorabilia, and photographs. The general files, minutes, and reports reflect the varied activities and interests of the League, including apportionment, court reform, education, and voting rights. The historical files contain photographs, printed materials, and memorabilia, filed chronologically. Also included are the periodicals and publications of the League, scrapbooks arranged chronologically, and "Mailbooks", or volumes of mimeographed reports and announcements which were sent to branches and board members. Among the major correspondentrs are: Thomas E. Dewey, Herbert H. Hehman, Nelson A. Rockefeller, Franklin D. Roosevelt, and Alfred Smith