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Correspondence, manuscripts, photographs, and printed materials of Sypher, reflecting his interest in A.C. Swinburne and in the Estonian poet, Aleksis Rannit. Correspondents include Joseph Hume, Ted Joans, Aleksis Rannit, Enid Starkie, and Algernon Charles Swinburne. There are additional materials on Africa, the Mina dialect in Togo, and the Sypher and related families of New York State.

Primarily oil portraits of 18th century literary figures. There are also engravings, and pen and ink and pencil sketches. Among the literary figures are portraits of Samuel Butler, Lord Byron, Thomas Carlyle; Colley Cibber; Charles Dickens; John Evelyn; John Foxe; David Garrick; Thomas Gray; Charles Lamb; Sir Thomas More; Sir Walter Raleigh; Samuel Richardson; Richard B. Sheridan; Alfred, Lord Tennyson; William M. Thackeray; and others. There is also a portrait by Blanche Ames of George A. Plimpton. Among the artists represented in the collection are James Maubert, Frederick Sandys, and William Hogarth (attrib.)

One letter from Walt Whitman to Alfred Lord Tennyson and three manuscripts by Whitman, one of which is a photostatic copy, several pieces of memorabilia and printed material by and about Whitman. The printed material includes newspaper clippings, pamphlets, periodical articles, illustrations, portraits of Whitman and publications of the Walt Whitman Birthplace Association