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The collection consiste of correspondence, memoranda, reports, bulletins, clippings, photographs, awards, and printed material. The files, arranged by genre and topic and reflect her philanthropic and legislative work in the areas of health, specifically cancer, heart disease, and mental health. Her civic and legislative work is covered in detail, as well as her private interests and activities.

Letters, invitations, documents, page proofs, photographs, lithographs, and books of Rosenman. Letters from political acquaintances including Benjamin Cardozo and W. Averell Harriman, to Rosenman and his wife, Dorothy, one letter by Henry Clay to H. Shaw 23 Sept. 1826 collected by Rosenman, invitations to official social functions, two sets of proofs for political pamphlets written by Rosenman on behalf of New York Governor Alfred E. Smith, photographic and lithographic portraits of political acquaintances signed and inscribed to Rosenman, including those of Dwight D. Eisenhower, W. Averell Harriman, Franklin D. Roosevelt, and Harry S. Truman. Other correspondents include Charles A. Beard, Louis D. Brandeis, Dwight D. Eisenhower, and Wendell Willkie. Also, thirteen books dealing with the Roosevelt administration signed and inscribed by the authors.

Correspondence, notes, articles, reports, and speeches of Gildersleeve, including materials relating to the United Nations Conference in San Francisco, 1945, the Dumbarton Oaks Conference, the International Federation of University Women, the American Association of University Women, the American Council on Education, and the Near East College Association. The most note-worthy item in the collection is a letter from President Franklin D. Roosevelt, appointing Dean Gildersleeve to serve as a member of the U.S. Delegation to the Charter Conference of the United Nations. The collection also contains some material relating to Barnard College affairs.