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This collection of letters, manuscripts, autographs, and illustrations of English and American authors and statesmen was assembled by George Dunlop. Many of the letters relate to Robert Burns and to the Burns country of Ayrshire. Among the early items are letters from Robert Burns, Samuel Johnson, Hester Thrale Piozzi, Edgar Allan Poe, and Abraham Lincoln.

Correspondence, manuscripts of poems, and manuscripts of lectures by Benjamin. The correspondence consists of original letters of Benjamin, typescript and photostatic copies of Benjamin letters in other libraries, and letters to Benjamin from some of his literary contemporaries including Paul Hamilton Hayne, Willis Gaylord Clark, John Lothrop Motley, and Fitz-Greene Halleck. Many of the letters relate to Park Benjamin's lecture tours. There are other family letters and many documents relating to the Benjamin family,and two letterbooks of John Lothrop Motley. Also, a large amount of genealogical material of the Benjamin family, and its related families from the 16th century to the present day. There are also financial records, monographs, clippings, and photographs.