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The George A. Plimpton Papers consist largely of personal and professional correspondence, financial and real estate records, personal diaries and albums, writings, and lectures produced by or for George Arthur Plimpton. But the Papers also contains not only the correspondence and records of Plimpton's colleagues at Ginn and Company, the publishing house that Plimpton led for decades, but also correspondence and records relating to the dozens of other institutions and organizations that Plimpton helped lead. In addition to extensive correspondence relating to Plimpton's collecting of rare books, manuscripts, and historical artifacts, the Papers also contain such diverse items as autographs of presidents, handwriting specimens, studies of medieval manuscripts, and documents relating to the American slave trade.

The Near East College Association formed in 1927 to combine financial and administrative work in a joint office for efficiency in management and to help raise endowment funds for institutions from Greece, Turkey, Lebanon, Syria, Bulgaria, and Iraq. The collection contains administrative records, correspondence, publications, and records related to partner institutions.

This collection contains records related to the American Committee for Armenian and Syrian Relief, established in 1915 to respond to the Armenian Genocide, and incorporated through an Act of Congress and renamed Near East Relief in 1919.