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Approximately 12,000 letters to Allan Nevins from various correspondents including James Truslow Adams, Franklin Delano Roosevelt, Harry S. Truman, Willa Cather, Frances Folsom Cleveland, Van Wyck Brooks, Robert Frost, Newton D. Baker, Archibald MacLeish, John D. Rockefeller, Jr., Carl Sandburg, and Henry Wallace; notes and typescripts for Nevins' books including Emergence of Lincoln, The Ordeal of Democracy, Rockefeller, and History and Historians, with notes by editor Ray A. Billington; miscellaneous transcripts, clippings, newspapers, and photographs. Also, autograph letters and manuscripts by presidents, Civil War figures, financiers, politicians, and authors. There are also the Brand Whitlock World War I Diaries and letters to him by such people as Herbert Hoover, Gen. John J. Pershing, and others.

Correspondence, scripts, manuscripts, and reports regarding his activities in the American radio and film industries. Included are papers regarding projects for the United State Government, the Indian film industry, various television and radio networks, and private ventures. Also included is material regarding the Center for Mass Communications of Columbia University, in which Barnouw figured prominently and files for the books he has written.

Correspondence, manuscripts, notes, documents, subject files, photographs, art works, and printed materials. This collection covers the entire span of his life, although by far the greatest part relates to his activities as a professor from the 1930s to the 1960s. Among the correspondents are many important figures in American Russian studies or Columbia University; there are also many letters from his wife, Clemens T. Robinson, and Lewis Mumford. Manuscripts by Robinson include his "Rural Russia under the Old Regime" lectures, notes, speeches and essays, and also miscellaneous pieces (essays, reviews, poems, stories, plays, etc.) that he wrote while he was an aspiring young journalist and writer in the 1910s and 1920s. Manuscripts by others consist of student theses, papers, books and reports that were given him for review or comment. Subject files deal with such topics as his service in World War I; Columbia University (especially the Libraries and the History Department); and various aspects of academic life and Russian studies. Almost nothing in the collection has any bearing on his government service during World War II; items from the war years concern personal affairs or scholarship. There are photographs of Robinson and his wife; family photographs from the late 19th and early 20th centuries; and Russian scenes. Art works include items by Clemens T. Robinson. Among the printed materials are two books inscribed by Mumford to Robinson.

Correspondence and manuscripts of Van Doren, consisting of letters, poems, short stories, novels, plays, radio broadcast transcripts ("Invitation to Learning"), diaries, critical works, proofs, and printed works. Correspondents include Louise Bogan, Philip Booth, Babette Deutsch, Richard Eberhart, T.S. Eliot, John Gould Fletcher, Herbert Gorman, E.W. Howe, Robinson Jeffers, Archibald MacLeish, Louis MacNeice, Edgar Lee Masters, Lewis Mumford, Hyam Plutzik, Allen Tate, and Louis Zukovsky. Also, extensive correspondence with Robert Lax and Thomas Merton, as well as manuscripts by these two authors.

Correspondence, playscripts, screenplays, scenarios, short stories, and other manuscripts, drafts, photocopies, contracts and other documents, tearsheets, clippings, and other materials relating to his career as a screenwriter, playwright, and author of short stories. Correspondence with friends, students, admirers, and professional colleagues concern his teaching, playwriting, films, articles, photography, and literary topics. There are also two groups of letters from students and readers about his textbook, "The Human Nature of Playwriting" (1949). Among the cataloged correspondence are William Gibson, MacKinlay Kantor, Anna Louise Strong, Louis Untermeyer, and Carl Van Doren. Included are manuscripts, drafts, or photocopies of almost all his films, plays, and short stories, such as playscripts and drafts of his plays, "The Jazz Singer" (1922), "Skylark" (1939), "Jason" (1942), and others; screenplays and scenarios, many in photocopy, of "Trouble in Paradise" (1932), "The Merry Widow" (1934), "The Shop Aroung the Corner" (1940), "Suspicion" (1941), "Heaven Can Wait" (1943), and many other films; and manuscripts, drafts, tearsheets, and printed copies of his short stories and articles of film and television criticism. There are also many clippings and reviews, programs, and other printed materials about his plays and films.