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Minutes, correspondence, annual reports, press releases, financial records, photographs, memorabilia, audiovisual, digital and printed materials document the philanthropic activities and administration of the Carnegie Corporation of New York. The collection is actively growing, primarily through regular document transfers from the Carnegie Corporation of New York. Andrew Carnegie's biographical information and personal philanthropic activity can be found in Series VII. In addition, his pre-1911 gifts, most notably his donations for libraries and church organs, can be found on microfilm (Series II), in the Home Trust Company Records (VI.A), and Financial Record Books (I.C.1). Grant files (Series III.A), which comprise the bulk of the collection) provide information on projects and institutions founded, endowed or supported by the Corporation. The Special Initiatives series (Series IV) contains the records of task forces, commissions and councils, formed by the Corporation mostly during the 1970s, 1980s, and 1990s to address specific issues. The Corporation's records include those of other Carnegie philanthropic organizations (Series VI), including the Carnegie Foundation for the Advancement of Teaching and the Home Trust Company, both of which shared staff, officers, and office space with the Corporation for a period of time.

Correspondence, memoranda, and legal and financial documents of Keppel. The files deal largely with Keppel's personal and professional life during his tenure as President of the Carnegie Corporation, and also include some files from his years as Newton D. Baker's Third Assistant Secretary of War, and as Dean of Columbia College. There are extensive files of correspondence from and to Keppel's parents and children, as well as files concerning his activities in organizations such as the Century and Columbia University Clubs. The letters from friends and business associates concern American education, politics, business, and cultural life, particularly in the New York metropolitan area, from 1900 to 1943.