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Papers of the Jay family and of those families related to the Jay family, including Bruen, Butterworth, Chapman, Clarkson, Dawson, Du Bois, Field, Iselin, McVickar, Mortimer, O'Kill, Pellew, Pierrepont, Prime, Robinson, Schieffelin, Von Schweinitz, Sedgwick, and Wurts. In addition to family and personal matters, the correspondence deals with anti-slavery, New York State civil service, repeal of the Missouri Compromise, the Civil War, the Blair Bill, international affairs, and New York City and State politics and government. There are letters from numerous prominent persons including George Bancroft, F.A.P. Barnard, Bismarck, William Cullen Bryant, Aaron Burr, James Fenimore Cooper, Ralph Waldo Emerson, Hamilton Fish, Albert Gallatin, Horace Greeley, Nathaniel Hawthorne, Oliver Wendell Holmes, Washington Irving, Frances Anne Kemble, Jenny Lind, Henry W. Longfellow, Seth Low, James Russell Lowell, John Stuart Mill, Alice Duer Miller, Clement Clarke Moore, J.P. Morgan, Thomas Nast, Commodore Matthew Perry, Franklin D. Roosevelt, Theodore Roosevelt, Elihu Root, Carl Schurz, William H. Seward, William T. Sherman, Charles Sumner, and John Greenleaf Whittier.

Letters written to Mrs. Josephine Sophie White Griffing relating to her interests in the emancipation of African-Americans, temperance, and woman's suffrage. It is evident that the letters have been preserved selectively from Mrs. Griffing's papers, all of them being from well-known contemporaries. Correspondents include Frederick Douglass, Charles Sumner, Horace Greeley, Henry Ward Beecher, Anna Dickinson, Lucretia Mott, William H. Seward, and John Greenleaf Whittier. Many of the letters relate to her efforts to have prominent people give lectures in support of women's suffrage. Also, a scrapbook of clippings about Mrs. Griffing's life and activities and the autograph book of George T. Driggs, a relative, which contains the signatures of prominent political and military figures, particularly members of Congress, during the late 1860s.

Correspondence, manuscripts of poems, and manuscripts of lectures by Benjamin. The correspondence consists of original letters of Benjamin, typescript and photostatic copies of Benjamin letters in other libraries, and letters to Benjamin from some of his literary contemporaries including Paul Hamilton Hayne, Willis Gaylord Clark, John Lothrop Motley, and Fitz-Greene Halleck. Many of the letters relate to Park Benjamin's lecture tours. There are other family letters and many documents relating to the Benjamin family,and two letterbooks of John Lothrop Motley. Also, a large amount of genealogical material of the Benjamin family, and its related families from the 16th century to the present day. There are also financial records, monographs, clippings, and photographs.