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Minutes, correspondence, annual reports, press releases, financial records, photographs, memorabilia, audiovisual, digital and printed materials document the philanthropic activities and administration of the Carnegie Corporation of New York. The collection is actively growing, primarily through regular document transfers from the Carnegie Corporation of New York. Andrew Carnegie's biographical information and personal philanthropic activity can be found in Series VII. In addition, his pre-1911 gifts, most notably his donations for libraries and church organs, can be found on microfilm (Series II), in the Home Trust Company Records (VI.A), and Financial Record Books (I.C.1). Grant files (Series III.A), which comprise the bulk of the collection) provide information on projects and institutions founded, endowed or supported by the Corporation. The Special Initiatives series (Series IV) contains the records of task forces, commissions and councils, formed by the Corporation mostly during the 1970s, 1980s, and 1990s to address specific issues. The Corporation's records include those of other Carnegie philanthropic organizations (Series VI), including the Carnegie Foundation for the Advancement of Teaching and the Home Trust Company, both of which shared staff, officers, and office space with the Corporation for a period of time.

Correspondence, speeches, reports, testimony, press releases, and articles of Young. The files document Young's leadership in many social welfare and civil rights organizations, as well as his activities as a columnist and speaker. Cataloged correspondents include Robert F. Kennedy, Lyndon B. Johnson, Hubert H. Humphrey, Martin Luther King, Jr., Coretta Scott King, Roy Wilkins, and John W. Gardner.

Correspondence, memoranda, notes, speeches, scientific data, photographs and printed material. Half of the collection relates to McGill's research and writing in the fields of experimental and mathematical psychology, particularly in the psychology of perception, and contains drafts of papers, notes, class materials and works by others. Also included are files relating to McGill's chairmanship of the Carnegie Commission on the Future of Public Broadcasting, files pertaining to his participation on the New York State Special Advisory Panel on Medical Malpractice, and some papers from his chairmanship of the psychology department, and later chancellorship, of the University of California, San Diego. Some personal correspondence and documents are also included. Among the cataloged correspondence are John W. Gardiner, Edward M. Kennedy, Margaret Mead, Daniel Patrick Moynihan, Jonas Salk, and Beverly Sills