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Correspondence, manuscripts, diaries, notebooks, and publications. The many manuscripts reflect Barzun's interest in poetry, literature and political affairs. The collection also contains materials for the journal, Art et Action which Barzun helped to found; lecture notes, 1933-1952; and a few items pertaining to Filippo Tommaso Marinetti and the Futurists. There are some Barzun family papers, as well. The correspondents are primarily French and American authors including André Breton, Katherine Dreier, Marcel Duchamp, Georges Duhamel, Albert Gleizes, Ivan Goll, Harriet Monroe, Ezra Pound, Pierre Reverdy, Edgar Varèse, Gabriel d'Annunzio, and Felippo Tommaso Marinetti.

The collection includes the original manuscript of "Surrender on Demand", Mr. Fry's account of his wartime experiences, which was later rewritten for young readers as "Assignment Rescue" (New York, Four Winds Press, 1968). Among the correspondents represented in the collection are Marc Chagall, Jacques Lipchitz, Roger Baldwin, Norman Thomas, J. Edgar Hoover, and Herman Wouk. In addition to the material relating to the Emergency Relief Committee (later known as the International Rescue Committee), the collection includes correspondence and papers concerning Fry's work as a writer on foreign affairs as well as copies of his books.