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The surviving files of official correspondence, reports, documents, and printed materials of King's College from 1750 to 1784 and Columbia College from 1785 to 1890, as well as Columbia University up to 1964. The King's College era materials include grants, deeds, indentures, lists of governors, leases, accounts, etc. The Columbia College era papers commence with documentation regarding the attempts to revive the college at the end of the American Revolution. In the later period these papers primarily supplement and document the minutes of the meetings of the Board of Governors and the Board of Trustees. Much material was destroyed and scattered in the late 19th century leaving this collection quite incomplete.

This collection is composed of the general files of Columbia College's Dean's Office, the minutes of Columbia College committees and the correspondence of Columbia College administrative officers during the years 1892 through 2019. A review of this collection allows researchers to gain insights into the interaction of Columbia College faculty and administrators with students, fellow faculty members, parents of students, and administrators of other colleges.

Established in 1965 by Columbia University, the Double Discovery Center (DDC) provides educational programs and services to low income and first generation college-bound junior high and high school students in New York City. The DDC is one of the oldest Upward Bound programs in the United States. The collection contains the records of the DDC from 1965 to 2005, including student files and materials documenting the DDC's primary programs, Upward Bound and Talent Search.

This collection consists of correspondence, translated letters, memoranda, and reports related to Inter-University Committee on Travel Grants activities, an organization that facilitated the exchange of students and scholars between American universities and the Soviet Union.