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Minutes, correspondence, annual reports, press releases, financial records, photographs, memorabilia, audiovisual, digital and printed materials document the philanthropic activities and administration of the Carnegie Corporation of New York. The collection is actively growing, primarily through regular document transfers from the Carnegie Corporation of New York. Andrew Carnegie's biographical information and personal philanthropic activity can be found in Series VII. In addition, his pre-1911 gifts, most notably his donations for libraries and church organs, can be found on microfilm (Series II), in the Home Trust Company Records (VI.A), and Financial Record Books (I.C.1). Grant files (Series III.A), which comprise the bulk of the collection) provide information on projects and institutions founded, endowed or supported by the Corporation. The Special Initiatives series (Series IV) contains the records of task forces, commissions and councils, formed by the Corporation mostly during the 1970s, 1980s, and 1990s to address specific issues. The Corporation's records include those of other Carnegie philanthropic organizations (Series VI), including the Carnegie Foundation for the Advancement of Teaching and the Home Trust Company, both of which shared staff, officers, and office space with the Corporation for a period of time.

Correspondence of Williamson covering his college years and his positions at Bryn Mawr College, the New York Public Library, the Carnegie Foundation, and the Rockefeller Foundation. A significant portion of Williamson's Columbia University correspondence and memoranda is addressed to or related to Roger Howson, University Librarian from 1926 to 1940. The manuscripts, chiefly typescripts, are concerned with library science and educational topics. Also, clippings and pamphlet files with some related correspondence and typescripts dealing with education and particularly the use of television as a teaching aid.