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Most of the collection consists of letters to Golśteĭn; there are some as well to her second husband, Vladimir A. Gol'shtein. The materials reflect Gol'shtein ties to Russian liberalism and populism and also to both French and Russian art and literature. There are groups of cataloged letters from Renʹe Arcos (15), Mykhailo Drahomaniv (52), Andrʹe Fontainas (31), Renʹe Ghil (32), Viacheslav Ivanov (17), Petr Lavrov (49), Vladimir Vernadskii (20), and Maksimilian Voloshin (29). There are also items by Jurgis Baltrušaitis, Henri Martin Barzun, Henri Bergson, Ivan Bunin, Sergei Diagilev, Paul Fort, Vladislav Khodasevich, Aristide Maillol, and Odilon Redon. Manuscripts are chiefly by Golśhteĭn, and include her memoirs on Drahomaniv. There are also poems by Voloshin and by Konstantin Bal'mont. Subject files deal with such topics as the Russian famine of 1891-92 and the Russian Liberation Committee at the time of the Civil War. There is a copy of Gol'shtein's book, "Serf Life in Russia."

The papers consist of correspondence, manuscripts, documents, original art works, bibliographic notes and material on exhibitions. There are letters from Aleksandr Benois, Mikhail Chekhov, Fedor Komissarzhevskiĭ, Georgiĭ Lukomskiĭ, Nikolaĭ Medtner, Vladimir Nabokov and Aleksandra Tolstai︠a︡, and one letter each from Ivan Bunin, Mikhail Fokin, Tyrone Guthrie, Sok Hurok and Serge Kusevit︠s︡kiĭ. The manuscripts include essays by Dobuzhinskiĭ on such topics as the Mir Iskusstva group, Pushkin's illustrations, Aleksandr Blok, Kuzḿa Petrov-Vodkin and Josʹe-Maria Sert. There are original art works (pen and ink, goache, etc.) relating to his artistic and theatrical productions. Also included are photographs of Russian scenes, apparently from before World War I.