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The collection documents the scholarship and writing of John Eugene Unterecker, a poet, biographer of the poet Hart Crane, and professor of English. The majority of the collection is composed of correspondence and manuscripts. Materials date from 1961 to 1987.

Correspondence and manuscripts of Van Doren, consisting of letters, poems, short stories, novels, plays, radio broadcast transcripts ("Invitation to Learning"), diaries, critical works, proofs, and printed works. Correspondents include Louise Bogan, Philip Booth, Babette Deutsch, Richard Eberhart, T.S. Eliot, John Gould Fletcher, Herbert Gorman, E.W. Howe, Robinson Jeffers, Archibald MacLeish, Louis MacNeice, Edgar Lee Masters, Lewis Mumford, Hyam Plutzik, Allen Tate, and Louis Zukovsky. Also, extensive correspondence with Robert Lax and Thomas Merton, as well as manuscripts by these two authors.