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Papers of Smedley, including correspondence, memoranda, manuscripts, and printed materials about the United Nations, national politics and elections, and civic organizations in New York City and in Connecticut. Correspondents include Hubert Humphrey, John F. Kennedy, and Bertrand Russell.

Correspondence, manuscripts, dispatches, documents, clippings and other printed materials concerning his career as an editor and correspondent for the New York Herald Tribune in Moscow, Berlin and New York, as a staff member of the Institute of Pacific Relations from 1932 to 1934, as deputy director in the Office of War Information overseas branch, 1941-44, as an owner and editor of the New York Star, 1948-49, as an instructor in communications at Sarah Lawrence College, 1950-1951, as a book editor at Simon and Schuster, Publishers, 1951-1970, and as an author and translator.

Correspondence, manuscripts, diaries, drafts, notes, documents, proofs, clippings, printed books, and other related materials. There are typescript drafts, proofs, related correspondence,, and printed copies of each of her books; typescript and tearsheets of her short stories, novelettes, and playscripts; correspondence with readers, agents, and publishers, and files for her promotional work at Time-Life, her newspapare and magazine columns, and her other interests; her daily appointment books; and her financial records. Among the cataloged correspondence are: Roger Nash Baldwin, Moss Hart, Hubert H. Humphrey, Ernest Jones, Clare Boothe and Henry Luce, Thomas Mann, Jo Mielziner, and Dorothy Thompson.