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Minutes, correspondence, annual reports, press releases, financial records, photographs, memorabilia, audiovisual, digital and printed materials document the philanthropic activities and administration of the Carnegie Corporation of New York. The collection is actively growing, primarily through regular document transfers from the Carnegie Corporation of New York. Andrew Carnegie's biographical information and personal philanthropic activity can be found in Series VII. In addition, his pre-1911 gifts, most notably his donations for libraries and church organs, can be found on microfilm (Series II), in the Home Trust Company Records (VI.A), and Financial Record Books (I.C.1). Grant files (Series III.A), which comprise the bulk of the collection) provide information on projects and institutions founded, endowed or supported by the Corporation. The Special Initiatives series (Series IV) contains the records of task forces, commissions and councils, formed by the Corporation mostly during the 1970s, 1980s, and 1990s to address specific issues. The Corporation's records include those of other Carnegie philanthropic organizations (Series VI), including the Carnegie Foundation for the Advancement of Teaching and the Home Trust Company, both of which shared staff, officers, and office space with the Corporation for a period of time.

Architectural drawings and specifications for Codman's projects, circa 1890s-1930s, including the Martha Codman house in Washington, D.C.; alterations for Edith Wharton and her husband at their three residences, the Mount in Lenox, Mass., Land's End in Newport, R.I., and their Park Avenue home in New York City; work for the Thayer family of Boston, Mass., specifically Nathaniel Thayer's three homes in Boston, Lancaster, Mass., and Newport, R.I. ("Edgemere"), Bernard Thayer's Beacon Hill houyse in Boston, and Eugene Van Rensselaer Thayer's two houses in Boston and Lancaster, Mass.; the Lucy Dahlgren house in New York City; the Archer M. Huntington house on Fifth Avenue in New York City; interior design for John D. Rockefeller in his house "Kykuit" at Pocantico Hills, N.Y.; interior design work for the Vanderbilt family including Cornelius Vanderbilt's "Breakers" at Newport, R.I. and Frederick William Vanderbilt's mansion in Hyde Park, N.Y. and his house on Fifth Avenue in New York City; Oliver Ames' mansion at Pride's Crossing, Beverly, Mass., and his house in Boston; and interior decoration and alterations for Codman's own homes in Newport, R.I. and Roslyn, N.Y. and his villa in France, "La Leopolda", at Villefranche-sur-Mer. Also, lists, descriptions, and postcards of French chateaux, with related correspondence, circa 1900s-1930s, relating to Codman's bibliography on the chateaux of France; and miscellaneous lists of houses in England and France, correspondence, and printed material.

Architectural drawings and photographs of architectural drawings with some related correspondence of residential and public buildings, churches, libraries, theaters, monuments, and bridges including: the Henry Hudson Bridge, Triborough Bridge, and the Manhattan Bridge in New York; Edward Henry Harriman's Arden House in Harriman, N.Y.; the Alfred I. Dupont mansion in Roslyn, N.Y.; the David A. Reed house in Washington, D.C.; the reconstruction of the Grand Army Plaza in New York City; the Memorial Amphitheater for Arlington National Cemetery; and various bicentennial buildings for Yale University. Of note are drawings of the grounds, details of buildings, and furniture for the New York Public Library, 1908-1909.