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Levi's correspondence with his wife, Alice Fries Levi, letters of other family members, his diaries, his school and college notebooks and papers, awards and medals, and personal photographs. The earliest item in the collection is a scrapbook kept by his father, Albert A. Levi, in San Francisco, 1862.

Letters chiefly written to James Duane Livingston, 1787-1893, and documents, 1785-1915. The letters relate to the Livingston family affairs, principally matters concerning the family estate "Livingston Manor" and they are most numerous for the period 1787 to 1840. There are, however, two informative letters dated 1858 and 1860 from members of the family situated in San Francisco. The documents consist of wills, surveys, checks, notes, accounts, and similar papers. Also, a quantity of miscellaneous clippings, mementos, and the like.