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The collection consists primarily of correspondence, photographs, project records, architectural drawings, legal documents, periodicals, news clippings and exhibition materials. The material held in this collection relates to architectural projects for Edgar J. Kaufmann by Frank Lloyd Wright, and the bulk of the material relates to Kaufmann's home, Fallingwater, at Bear Run, Pennsylvania. The collection documents the professional and personal relationship between the Kaufmann family and Wright, from the 1930s until the years preceding Wright's death in 1959.

Professional and personal files including Armstrong's correspondence with professional associations, other engineers, and friends, his research notes, circuit diagrams, lectures, articles, legal papers, and other related materials. Of his many inventions and developments, the most important are: 1) the regenerative or feedback circuit, 1912, the first amplified radio reception, 2) the superheterodyne circuit, 1918, the basis of modern radio and radar, 3) superregeneration, 1922, a very simple, high-power receiver now used in emergency mobile service, and 4) frequency modulation - FM, 1933, static-free radio reception of high fidelity. More than half the files concern his many lawsuits, primarily with Radio Corporation of America, over infringement of the Armstrong patents. Litigation continued until 1967. Other files deal with his work in the Marcellus Hartley Research Laboratory at Columbia University, 1913-1935, and with the American Expeditionary Forces in France during World War I, his Air Force contracts for communications development, Army research during World War II, the Radio Club of America, the Institute of Radio Engineers, FM development at his radio station at Alpine, N.J., the use of FM in television, his involvement in Federal Communications Commission hearings and legislation, and his work with the Zenith Radio Corporation. Also, letters to H.J. Round

The collection includes correspondence from Konstantin Balḿont, Nikolaĭ Evreĭnov, Zinaida Gippius, Georgiĭ Grebenshchikov, Vasiliĭ Maklakov, Sergeĭ Potresov and Nadezhda Teffi. There is one letter each from Boris Bakhmeteff, Vera Bunina, Aleksandr Grechaninov, Aleksandr Kuprin and Alekseĭ Tolstoĭ. The manuscripts include poems and a play scenario by Nadezhda Teffi as well as Roshchina-Insarova's autobiographical essays and article about Sergeĭ Lifar.́ In addition, there are three scrapbooks containing clippings and programs of Roshchina-Insarova's performances, and approximately 40 photographs of her.

This collection includes nine letters of Ralph Waldo Emerson as well as letters of Louis Agassiz, Amos Bronson Alcott, Oliver Wendell Holmes, Sr., Henry Wadsworth Longfellow, James Russell Lowell, John Lothrop Motley, Charles Sumner, and John Greenleaf Whittier. In addition, there are two incomplete manuscripts by Emerson and one document from the Liverpool Custom-house signed by Nathaniel Hawthorne as Consul for the United States. The collection also includes the corrected typescript, index, and page and galley proofs for Thomas Franklin Currier, A BIBLIOGRAPHY OF OLIVER WENDELL HOLMES (New York, 1953) which was edited by Professor Tilton. Also, some early correspondence and photographs of the Tilton family and friends. There are letters from the actors Annie Louise Ames, Richard J. Dillon, and Hans L. Meery to Tilton's grandfather, Bernard Paul Verne, as well as photographs, tintypes, and daguerreotypes of the Verne family and friends.

Papers include correspondence, manuscripts, documents, photographs, subject files, and printed materials. The extensive correspondence relates to Mogilat's personal and professional activities and includes letters from many of her students and colleagues. Correspondents include Gleb Struve, Alexandra Tolstoy and Boris Unbegaun. Of special interest are letters by her first husband Baron von Taube, written from the front during World War I, and correspondence with various Russian acqaintances about the Soviet Union in the 1920s and 1930s in which they describe life in a communal apartment, and plans to rescue friends who have been arrested. Subject files concern Columbia's Russkiĭ Kruzhok and the Avtonomoff method of teaching Russian to Americans. There are letters, photographs, concert programs and music of Russian emigre composer and pianist Ariadna Mikeshina. Manuscripts are by various persons; most are by John Paul Mihaly, who had been Mogilat's student. There is also a manuscript of translations by Clarence Manning, "Four Poems by Blok." Documents and photographs concern Mogilat and her family, both before and after emigration. Printed materials consist mostly of off-prints of articles by Clarence Manning and others, primarily on literary topics. There are also books, mimeographed materials, periodicals, and clippings.