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Materials comprise correspondence, subject files, organizational files, course materials, speeches, notes, manuscripts, publications and reviews, and printed materials.

The records include annual reports, correspondence, memos, minutes, program files, news clippings, administrative records and photographs. They document the agency from its origins in a committee led by the Lenox Hill Neighborhood Association to its work during the 1990s providing social services to thousands of East Side residents. The founding and early history of the Stanley M. Isaacs Neighborhood Center are best documented by minutes in Series II, showing the collaboration between the New York City Housing Authority and the Lenox Hill Neighborhood Association to establish the agency. They also offer the most comprehensive view of administrative, fundraising and program decisions from the early years to the 1990s. This series is supplemented by architectural drawings and plans for the community center in Series VI. Program records in Series V focus on the period 1980-90, with a few items from the 1960s and '70s. The agency's fundraising efforts are documented in Series III, which includes correspondence with foundations and individuals, donor lists and committee files.

The Union Settlement Association Records document a century of the settlement's activities, and provide a unique view of the first wave of the settlement movement in America. They document social conditions, demographic change, political activity, philanthropy and social work in East Harlem with a strong emphasis on the urban renewal period of the 1950s and '60s. The records include: annual reports, board minutes and committee files, headworker and executive director files, program reports, community organization files, and visual materials such as photographs, maps and architectural drawings.

A collection of 1,200 essays on "New York's Future as I View It" written by high school students from the New York metropolitan area.