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Correspondence, minutes, reports, documents, scrapbooks, publications, memorabilia, and photographs. The general files, minutes, and reports reflect the varied activities and interests of the League, including apportionment, court reform, education, and voting rights. The historical files contain photographs, printed materials, and memorabilia, filed chronologically. Also included are the periodicals and publications of the League, scrapbooks arranged chronologically, and "Mailbooks", or volumes of mimeographed reports and announcements which were sent to branches and board members. Among the major correspondentrs are: Thomas E. Dewey, Herbert H. Hehman, Nelson A. Rockefeller, Franklin D. Roosevelt, and Alfred Smith

This collection contains copies of Butler's speeches delivered at Columbia University as well as at numerous other institutions from 1882 to 1947 during his tenure as president of the Industrial Education Association as well as Columbia University. While the speeches address a number of topics, they primarily focus on the state of America's higher educational system, potential educational reforms, and local and international American politics (particularly in relation to the Republican Party and war).