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This collection contains copies of Butler's speeches delivered at Columbia University as well as at numerous other institutions from 1882 to 1947 during his tenure as president of the Industrial Education Association as well as Columbia University. While the speeches address a number of topics, they primarily focus on the state of America's higher educational system, potential educational reforms, and local and international American politics (particularly in relation to the Republican Party and war).

Correspondence, diaries, documents, manuscripts, and printed materials. The collection consists chiefly of diaries, research materials, and his writings. Among the correspondents are: Mikhail Chekhov, Olga Chekhov, Roman Gul, Vladimir Ilin, Artur Luther, Sergei Melgunov, Bishop Serafim, Fedor Stepun, Ilia Surguchev, Alexandra Tolstoy, and Vladimir Zenzinov.