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This collection includes nine letters of Ralph Waldo Emerson as well as letters of Louis Agassiz, Amos Bronson Alcott, Oliver Wendell Holmes, Sr., Henry Wadsworth Longfellow, James Russell Lowell, John Lothrop Motley, Charles Sumner, and John Greenleaf Whittier. In addition, there are two incomplete manuscripts by Emerson and one document from the Liverpool Custom-house signed by Nathaniel Hawthorne as Consul for the United States. The collection also includes the corrected typescript, index, and page and galley proofs for Thomas Franklin Currier, A BIBLIOGRAPHY OF OLIVER WENDELL HOLMES (New York, 1953) which was edited by Professor Tilton. Also, some early correspondence and photographs of the Tilton family and friends. There are letters from the actors Annie Louise Ames, Richard J. Dillon, and Hans L. Meery to Tilton's grandfather, Bernard Paul Verne, as well as photographs, tintypes, and daguerreotypes of the Verne family and friends.

The collection contains correspondence with the authors, including contracts signed with authors as well as negotiations with the authors over various aspects of publishing their works; financial records documenting many aspects of the operation of Harper & Brothers, including royalties paid to authors, records of stock offerings and company reorganizations, and general ledgers which contain daily notes on all aspects of the operation of the business; book catalogues and trade lists; research materials collected by Eugene Exman for his history of Harper & Brothers; visual materials, from drawings and photographs of Harper's authors to colophon designs and an oil painting of the original Harper's building.

The editorial and production files of Pantheon Books from 1944 through 1968. The correspondence from authors, agents, and publishers is written to Kurt and Helen Wolff, Jacques Schiffrin, André Schiffrin, and the editors of the firm. The files document the publication of works by A. Alvarez, Georges Bernanos, Hermann Broch, Jacob Burckhardt, Albert Camus, William Demby, Eugene Ionesco, Karl Jaspers, Winifred Bryher, Jacques Maritain, Isamu Noguchi, José Ortega y Gasset, Pier Paolo Pasolini, Sir Herbert Read, Ben Shahn, and others.