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Correspondence, manuscripts, notes, notebooks, documents, photographs, course-related materials, and printed materials. The manuscripts include typescripts of Sykes' published and unpublished novels, monographs, plays, short stories, and articles. Among these are The Perennial Avant Garde, The Cool Millennium, and The Hidden Remnant. Sykes' notes and notebooks span the period from the early 1930s to 1980, and include preliminary ideas and sketches for his books, as well as autobiographical material. A small number of documents concern Sykes' wartime work in the U.S. Government Office of War Information. Course-related material including writings and correspondence of students taught by Sykes between 1962 and 1975 at the New School and as an adjunct professor at Columbia University. Printed materials consist of numerous reviews of Sykes' books, in addition to offprints and articles by Sykes. Included as well are printed materials about or connected with Sykes, offprints of articles inscribed to him, and many volumes from his library. The substantial correspondence series includes personal letters and correspondence with agents and publishers relating to his books. Correspondents include Harold Clurman, Aaron Copland, Lawrence Durrell, Georgia O'Keeffe, and Francis Steegmuller, as well as a number of Sykes' students. There is extensive correspondence between Sykes and the artist John Hartell from 1927 to 1983.

Correspondence, manuscripts, documents, oral histories, photographs, audio cassettes, and printed material. Family and personal correspondence; materials related to his secondary, college, and university education; materials related to his tenure at the National Council of the Protestant Church; business correspondence of St. Philip's Episcopal Church and the St. Philip's Community Service Council; bulletins of church services; drafts of sermons and speeches, as well as numerous audio-tapes; manuscripts and publications; correspondence related to the construction and on-going maintenance of several senior-citizen and other community housing; correspondence related to various community redevelopment initives and campaigns for affordable housing; materials related to college courses including oral histories for his Black Family Research project; photographs of St. Philip's Church and of activities of the St. Philip's Community Service Council.